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The mass spectrometric methods were first tested and were found to be adequate for the purpose of this work.

Moreover, it is possible to analyze the dye from a stroke directly from the paper (LDI-MS), so the sample preparation is minimized.

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The results show that the degradation of these dyes strongly depends on light fluence.

Humidity also increases degradation, which can be explained by the basicity of the paper.

The influence of heat on the degradation process was found to be rather weak.

It was also observed that the dyes from the ink strokes did not show significant degradation after one year of storage in the dark.

Therefore, it is important to understand the aging process of the different components found in ink.