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Although most of the important thermodynamic relations were known by 1895, they were seen as isolated equations, and had not yet been rationalized as a logical system, from which, given one relation, the rest could be derived.
Moreover, these relations were inexact, applying only to ideal chemical systems.
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These were two outstanding problems of theoretical thermodynamics.
In two long and ambitious theoretical papers in 19, Lewis tried to provide a solution.
Lewis successfully contributed to thermodynamics, photochemistry, and isotope separation, and is also known for his concept of acids and bases. As a professor, he incorporated thermodynamic principles into the chemistry curriculum and reformed chemical thermodynamics in a mathematically rigorous manner accessible to ordinary chemists.
After receiving his Ph D in chemistry from Harvard University and studying abroad in Germany and the Philippines, Lewis moved to California to teach chemistry at the University of California, Berkeley.
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There is evidence that he used the Nobel nominating and reporting procedures to block a Nobel Prize for Lewis in thermodynamics by nominating Lewis for the prize three times, and then using his position as a committee member to write negative reports.
After his stay in Nernst's lab, Lewis returned to Harvard in 1901 as an instructor for three more years.
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Most of Lewis’ lasting interests originated during his Harvard years.